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A Study on the Gaseous Benzene Removal Based on Adsorption onto the Cost-Effective and Environmentally Friendly Adsorbent

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Abstract

Removal of benzene is essential for human and environmental health because it has toxic and hazardous properties at various concentrations. Theseneed to be effectively eliminated with carbon-based adsorbents. PASACs, carbon-based adsorbents obtained from using the needles of Pseudotsuga menziesii, were produced by optimized HCl- and H2SO4-impregnated approaches. Regarding physicochemical structure, the optimized PASAC23 and PASAC35 with surface areas of 657 and 581 m2/g and total pore volumes of 0.36 and 0.32 cm3/g showed ideal temperatures of 800 °C. In order to investigate and compare internal benzene removal efficiency, PASAC23 and PASAC35 were studied separately. Initial concentrations were found to range from 5 to 500 mg/m3, and between 25 and 45 °C. The removal rate of benzene by PASAC23 and PASAC35 was 97 and 94% at low concentrations, respectively. While the highest capture amount for PASAC23 and PASAC35 was found to be at 25 °C with 141 and 116 mg/g, the adsorption capacity decreased to 102 and 90 mg/g at 45 °C. The holding capacity decreased between 22.41 and 27.66% due to increasing temperatures. After five cycles of PASAC23 and PASAC35 regeneration, we found that they could remove 62.37 and 58.46% of benzene, respectively. These results confirmed that PASAC23 is a promising environmentally adsorbent for effectively removing benzene with a competitive yield.

Date

2023-04-01

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air pollutants | environmental protection | gas treatment | reversible adsorption | sustainable porous carbons

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